Citation: Xibao Li, Yiyang Wan, Fang Deng, Yingtang Zhou, Pinghua Chen, Fan Dong, Jizhou Jiang. Advances in Z-scheme and S-scheme heterojunctions for photocatalytic and photoelectrocatalytic H₂O₂ production[J]. Chinese Chemical Letters, ;2025, 36(10): 111418. doi: 10.1016/j.cclet.2025.111418 shu

Advances in Z-scheme and S-scheme heterojunctions for photocatalytic and photoelectrocatalytic H₂O₂ production

Xibao Li ^{a, 1,} ,
Yiyang Wan ^{a, 1} ,
Fang Deng ^a ,
Yingtang Zhou ^b ,
Pinghua Chen ^a ,
Fan Dong ^{a, c} ,
Jizhou Jiang ^{d, *,}

a.
National-Local Joint Engineering Research Center of Heavy Metal Pollutants Control and Resource Utilization, Nanchang Hangkong University, Nanchang 330063, China
b.
Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control, National Engineering Research Center for Marine Aquaculture, Marine Science and Technology College, Zhejiang Ocean University, Zhoushan 316004, China
c.
Institute of Fundamental and Frontier Sciences, University of Electronic Science and Technology of China, Chengdu 611731, China
d.
School of Materials Science and Engineering, State Key Laboratory of Green and Efficient Development of Phosphorus Resources, Engineering Research Center of Phosphorus Resources Development and Utilization of Ministry of Education, Key Laboratory of Green Chemical Engineering Process of Ministry of Education, Hubei Key Laboratory of Plasma Chemistry and Advanced Materials, Novel Catalytic Materials of Hubei Engineering Research Center, Wuhan Institute of Technology, Wuhan 430205, China

lixibao@nchu.edu.cn

027wit@163.com

Received Date: 8 February 2025
Revised Date: 29 May 2025
Accepted Date: 6 June 2025
Available Online: 7 June 2025

Figures(20)

Photocatalytic and photoelectrocatalytic H₂O₂ production has been identified as a significant pathway within environmental pollution control, green energy, medical treatment, sterilization and disinfection. However, conventional single-material photocatalysts struggle to fulfill the stringent criteria of high efficiency, stability, cost-effectiveness, and responsiveness to visible light. The elevated recombination rates of photogenerated charge carriers, coupled with the suboptimal utilization of visible light, have collectively constrained the photocatalytic and photoelectrocatalytic H₂O₂ production. Heterojunction catalysts for the production of H₂O₂ has become a focal point of research. This review commences by elucidating the fundaments underlying the photocatalytic and photoelectrocatalytic H₂O₂ production. Subsequently, it delineates the distinctive electron transfer mechanisms of Z-scheme and S-scheme heterojunctions, which exhibit enhanced efficiency in the photocatalytic and photoelectrocatalytic H₂O₂ production, along with a summary of strategies for the improvement of photocatalyst and photoelectrocatalyst performance. Furthermore, this review also outlines the latest fabrication strategies, state-of-the-art in-situ characterization techniques, machine learning and density functional theory (DFT) simulations for Z-scheme or S-scheme catalysts for the photocatalytic and photoelectrocatalytic H₂O₂ production, and briefly describes the multifunctional applications in H₂O₂ production. Ultimately, the review contemplates the prospective developmental trajectories and application potential of these heterojunction configurations for the photocatalytic and photoelectrocatalytic H₂O₂ production.
- Photocatalytic and photoelectrocatalytic H₂O₂ production,
- Heterojunction,
- Electron transfer mechanisms,
- In-situ characterization,
- Machine learning
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Advances in Z-scheme and S-scheme heterojunctions for photocatalytic and photoelectrocatalytic H2O2 production

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通讯作者: 陈斌, bchen63@163.com

Advances in Z-scheme and S-scheme heterojunctions for photocatalytic and photoelectrocatalytic H₂O₂ production