Citation: Peng Gao, Hua Qiu, Huan Cheng, Zeyu Du, Xiao Chen, Xing Tan, Chenxi Cai, Qihong Zhang, Tong Yang, Nan Lyu, Qiufen Tu, Xingyi Li, Lei Lu, Nan Huang. Robust and versatile surface via in situ dynamic reassembly of polydopamine under strong alkaline conditions[J]. Chinese Chemical Letters, ;2025, 36(10): 110746. doi: 10.1016/j.cclet.2024.110746 shu

Robust and versatile surface via in situ dynamic reassembly of polydopamine under strong alkaline conditions

Peng Gao ^{a, b, 1} ,
Hua Qiu ^{b, c, 1} ,
Huan Cheng ^a ,
Zeyu Du ^b ,
Xiao Chen ^b ,
Xing Tan ^b ,
Chenxi Cai ^a ,
Qihong Zhang ^a ,
Tong Yang ^b ,
Nan Lyu ^b ,
Qiufen Tu ^b ,
Xingyi Li ^{d, *,} ,
Lei Lu ^{a, *,} ,
Nan Huang ^{b, e, *,}

a.
School and Hospital of Stomatology, Wenzhou Medical University, Wenzhou 325027, China
b.
Key Lab of Advanced Technology of Materials of Education Ministry, School of Materials Science and Engineering, Southwest Jiaotong University, Chengdu 610031, China
c.
Stomatologic Hospital and College, Key Laboratory of Oral Diseases Research of Anhui Province, Anhui Medical University, Hefei 230032, China
d.
National Engineering Research Center of Ophthalmology and Optometry, Eye Hospital, Wenzhou Medical University, Wenzhou 325027, China
e.
Guangzhou Nanchuang Mount Everest Company for Medical Science and Technology, Guangzhou 510530, China

lixingyi_1984@mail.eye.ac.cn

llu2@foxmail.com

huangnan1956@163.com

Received Date: 10 September 2024
Revised Date: 4 December 2024
Accepted Date: 9 December 2024
Available Online: 10 December 2024

Figures(4)

Polydopamine (PD) coating, one of the simplest and most versatile surface functionalization method faces challenges in terms of stability and reactivity. In this study, we propose an in situ dynamic reassembly approach to address these challenges. By immersing a pre-deposited PD coating in a strong alkaline solution containing poly(allylamine) hydrochloride (PAH), the dissociated PD oligomers undergo covalent crosslinking in situ, leading to the formation of a reconstructed PDPA coating enriched with stable amino groups through thorough crosslinking. The PDPA coating demonstrates superior chemical and mechanical stability compared to PD, while enhancing multifunctional properties and offering improved surface functional modification potential. The PDPA coating holds promise in materials science, biomedical engineering, and nanotechnology, enabling versatile surface modification and functionalization in extreme conditions.
- Polycatecholamine,
- Polydopamine,
- Material-independent coating,
- Dynamic reassembly,
- Covalently coating
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