Citation: Weikang Wang, Dajiang Mei, Shaoguo Wen, Jian Wang, Yuandong Wu. Complex coordinated functional groups: A great genes for nonlinear optical materials[J]. Chinese Chemical Letters, ;2022, 33(5): 2301-2315. doi: 10.1016/j.cclet.2021.11.089 shu

Complex coordinated functional groups: A great genes for nonlinear optical materials

Weikang Wang ^a ,
Dajiang Mei ^{a, c, *,} ,
Shaoguo Wen ^a ,
Jian Wang ^b ,
Yuandong Wu ^a

a.
College of Chemistry and Chemical Engineering, Shanghai University of Engineering Science, Shanghai 201620, China
b.
Department of Chemistry and Biochemistry, Wichita State University, Wichita, KS 67260, United States
c.
State Key Laboratory of Structural Chemistry, Fujian Institute of Research on the Structure of Matter, Chinese Academy of Sciences, Fuzhou 350002, China

meidajiang718@pku.edu.cn

Received Date: 13 September 2021
Revised Date: 21 October 2021
Accepted Date: 29 November 2021
Available Online: 4 December 2021

Figures(16)

Complex coordinated functional groups [MA_xB_y] (M = Central coordination element; A, B = P, O, S, Se, F, Cl, Br or I) are composed of different types of anions A, B jointly linked to the same central cation M, which are in high potential to tune the physical properties of materials, e.g., second-order susceptibility, energy gaps and birefringence. Recently, Compound containing complex coordinated functional groups have attracted great attention in the nonlinear optical (NLO) field and a large number of this type crystals exhibit promising NLO performance. However, the inherent relationship between ionic group structure and optical properties of complex coordinated NLO materials have not been systematically studied. This article systematically summarizes complex coordinated NLO materials in recent five years from the perspective of the internal relationship between crystal structure and optical properties. In addition, we propose the ideal combination and arrangement modes for structural building units, and also reveal the influence of complex coordinated functional groups [MA_xB_y] toward the NLO response, optical band gap and phase matching ability of complex coordinated NLO materials.
- Complex coordinated,
- Nonlinear optical,
- Second harmonic generation,
- Optical band gap,
- Structure-performance relationship
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沈阳化工大学材料科学与工程学院沈阳 110142