Citation: Conghui Wang, Ying-Ming Zhang, Haoran Li, Jin Zhang, Yu Zhou, Guoxing Liu, Xiufang Xu, Yu Liu. Synergistic activation of photoswitchable supramolecular assembly based on sulfonated crown ether and dithienylethene derivative[J]. Chinese Chemical Letters, ;2022, 33(5): 2447-2450. doi: 10.1016/j.cclet.2021.09.106 shu

Synergistic activation of photoswitchable supramolecular assembly based on sulfonated crown ether and dithienylethene derivative

Conghui Wang ^a ,
Ying-Ming Zhang ^a ,
Haoran Li ^b ,
Jin Zhang ^b ,
Yu Zhou ^a ,
Guoxing Liu ^c ,
Xiufang Xu ^a ,
Yu Liu ^{a, *,}

a.
College of Chemistry, State Key Laboratory of Elemento-Organic Chemistry, Nankai University, Tianjin 300071, China
b.
College of Computer Science, Nankai University, Tianjin 300350, China
c.
College of Sciences, Henan Agricultural University, Zhengzhou 450001, China

zzy@tjnu.edu.cn

cjli@shu.edu.cn

Received Date: 6 August 2021
Revised Date: 28 September 2021
Accepted Date: 30 September 2021
Available Online: 5 October 2021

Figures(4)

Conformational regulation among two or more distant sites is not only one of the main pathways to accomplish multiple tasks in complex biological systems but also represents a powerful strategy to obtain stimuli-responsive supramolecular nanoconstructs with tailored physicochemical performance. We herein report the fabrication of a photochromic supramolecular assembly, which can be synergistically activated by the conformational regulation with bis(4, 8-disulfonato-1, 5-naphtho)-32-crown-8 and then reversibly switched by the through-space communication between restricted stilbazolium salt and photochromic dithienylethene. This work demonstrates that the synergistic conformational modulation via intra- and intermolecular interactions can be developed as a generalizable approach to construct more advanced biomimetic nanomaterials.
- Supramolecular assembly,
- Crown ether,
- Photochromism,
- Energy transfer,
- Conformational regulation
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