Citation: Zengqiang Gao, Junjun Li, Zhicheng Zhang, Wenping Hu. Recent advances in carbon-based materials for electrochemical CO₂ reduction reaction[J]. Chinese Chemical Letters, ;2022, 33(5): 2270-2280. doi: 10.1016/j.cclet.2021.09.037 shu

Recent advances in carbon-based materials for electrochemical CO₂ reduction reaction

Tianjin Key Laboratory of Molecular Optoelectronic Sciences, Department of Chemistry, School of Science & Collaborative Innovation Center of Chemical Science and Engineering, Tianjin University, Tianjin 300072, China

zczhang19@tju.edu.cn

Received Date: 10 August 2021
Revised Date: 4 September 2021
Accepted Date: 9 September 2021
Available Online: 14 September 2021

Figures(13)

The increase of atmospheric CO₂ concentration has caused many environmental issues. Electrochemical CO₂ reduction reaction (CO₂RR) has been considered as a promising strategy to mitigate these challenges. The electrocatalysts with a low overpotential, high Faradaic efficiency, and excellent selectivity are of great significance for the CO₂RR. Carbon-based materials including metal-free carbon catalysts and metal-based carbon catalysts have shown great potential in the CO₂RR, owing to the tailorable porous structures, abundant natural resources, resistance to acids and bases, high-temperature stability, and environmental friendliness. In this review, various carbon materials including graphene, carbon nanotubes, quantum dots, porous carbon, and MOF-derived catalysts, etc., for the CO₂RR have been summarized. Particularly, recent progress in terms of the mechanism and pathway of CO₂ conversion has been comprehensively reviewed. Finally, the opportunities and challenges of carbon-based electrocatalysts for the CO₂RR are proposed.
- CO₂ reduction,
- Electrocatalysis,
- Carbon materials,
- Chemicals and fuels,
- Single-atom catalysts
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通讯作者: 陈斌, bchen63@163.com

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沈阳化工大学材料科学与工程学院沈阳 110142

Recent advances in carbon-based materials for electrochemical CO2 reduction reaction

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通讯作者: 陈斌, bchen63@163.com

Recent advances in carbon-based materials for electrochemical CO₂ reduction reaction