Citation: Fengqi Wang, Wenlong Zhang, Hongbin Wan, Chenxi Li, Wankai An, Xia Sheng, Xiaoyu Liang, Xiaopeng Wang, Yunlai Ren, Xin Zheng, Dongcan Lv, Yuchen Qin. Recent progress in advanced core-shell metal-based catalysts for electrochemical carbon dioxide reduction[J]. Chinese Chemical Letters, ;2022, 33(5): 2259-2269. doi: 10.1016/j.cclet.2021.08.074 shu

Recent progress in advanced core-shell metal-based catalysts for electrochemical carbon dioxide reduction

Fengqi Wang ^a ,
Wenlong Zhang ^a ,
Hongbin Wan ^b ,
Chenxi Li ^c ,
Wankai An ^a ,
Xia Sheng ^a ,
Xiaoyu Liang ^a ,
Xiaopeng Wang ^{a, *,} ,
Yunlai Ren ^a ,
Xin Zheng ^a ,
Dongcan Lv ^a ,
Yuchen Qin ^{a, *,}

a.
College of Sciences, Henan Agricultural University, Zhengzhou 450000, China
b.
Oilfield Technology Research Institute of Fengcheng Oilfield Operation Area, Xinjiang Oilfield Company, Karamay 834000, China
c.
College of Life Science, Chongqing Normal University, Chongqing 401331, China

xpwang@henau.edu.cn

qinyuchen@henau.edu.cn

Received Date: 14 June 2021
Revised Date: 14 July 2021
Accepted Date: 14 August 2021
Available Online: 19 August 2021

Figures(10)

Electrochemical carbon dioxide reduction (CO₂RR) plays an important role in solving the problem of high concentration of CO₂ in the atmosphere and realizing carbon cycle. Core-shell structure has many unique features including tandem catalysis, lattice strain effect, defect engineering, which exhibit great potential in electrocatalysis. In this review, we focus on the advanced core-shell metal-based catalysts (CMCs) for electrochemical CO₂RR. The recent progress of CMCs in electrocatalytic CO₂RR is described as the following aspects: (1) The mechanism of electrochemical CO₂RR and evaluation parameters of electrocatalyst performance, (2) preparation methods of core-shell metal catalysts and core-shell structural advantages and (3) advanced CMCs towards electrochemical CO₂RR. Finally, we make a brief conclusion and propose the opportunities and challenges in the field of electrochemical CO₂RR.
- CMCs,
- Electrochemical CO₂RR,
- Tandem catalysis,
- Lattice strain effect,
- Defect engineering
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沈阳化工大学材料科学与工程学院沈阳 110142