Citation: Huang Yan, Li Haifeng, He Xiaoxiao, Yang Xiaohai, Li Li, Liu Songyang, Zou Zhen, Wang Kemin, Liu Jianbo. Near-infrared photothermal release of hydrogen sulfide from nanocomposite hydrogels for anti-inflammation applications[J]. Chinese Chemical Letters, ;2020, 31(3): 787-791. doi: 10.1016/j.cclet.2019.05.025 shu

Near-infrared photothermal release of hydrogen sulfide from nanocomposite hydrogels for anti-inflammation applications

Huang Yan ^a ,
Li Haifeng ^a ,
He Xiaoxiao ^a ,
Yang Xiaohai ^a ,
Li Li ^a ,
Liu Songyang ^a ,
Zou Zhen ^b ,
Wang Kemin ^a,*, ,
Liu Jianbo ^a,*,

a.
State Key Laboratory of Chemo/Biosensing and Chemometrics, College of Chemistry and Chemical Engineering, Key Laboratory for Bio-Nanotechnology and Molecular Engineering of Hunan Province, Hunan University, Changsha 410082, China
b.
School of Chemistry and Food Engineering, Changsha University of Science and Technology, Changsha 410114, China

kmwang@hnu.edu.cn

liujianbo@hnu.edu.cn

Received Date: 12 April 2019
Revised Date: 28 April 2019
Accepted Date: 14 May 2019
Available Online: 18 May 2019

Figures(4)

A novel near-infrared light photothemal-activated H₂S-donating nanocomposite hydrogel was developed, through combination of a thermo-labile H₂S donor and photothermal nanoparticles in agarose hydrogel. The polyethylenimine dithiocarbamate polymer, a thermo-labile compound, was synthesized as a novel H₂S donor. The combination of a thermo-labile hydrogen sulfide donor and photothermal nanoparticles enabled the generation of H₂S in agarose hydrogel upon irradiation with near-infrared light. The ability to modulate the photoirradiation for controlled generation and spatiotemporally release of H₂S are its specific advantages. This photothermal spatiotemporally controlled H₂S-releasing strategy was successfully applied to anti-inflammation treatment in a rat model, demonstrating its utility as a novel H₂S-based therapeutic approach.
- Hydrogen sulfide,
- Near-infrared light,
- Photothermal transduction,
- Nanocomposite hydrogels,
- Anti-inflammation
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