Citation: Ding Yusen, Wang Yan, Su Yanjie, Yang Zhi, Liu Jiaqiang, Hua Xiaolin, Wei Hao. A novel channel-wall engineering strategy for two-dimensional cationic covalent organic frameworks: Microwave-assisted anion exchange and enhanced carbon dioxide capture[J]. Chinese Chemical Letters, ;2020, 31(1): 193-196. doi: 10.1016/j.cclet.2019.05.012 shu

A novel channel-wall engineering strategy for two-dimensional cationic covalent organic frameworks: Microwave-assisted anion exchange and enhanced carbon dioxide capture

Ding Yusen ^a,b,1 ,
Wang Yan ^a,b,1 ,
Su Yanjie ^a ,
Yang Zhi ^a ,
Liu Jiaqiang ^b,*, ,
Hua Xiaolin ^c,*, ,
Wei Hao ^a,*,

a.
Key Laboratorty for Thin Film and Microfabrication Technology of Ministry of Education, Shanghai Jiao Tong University, Shanghai 200240, China
b.
Department of Oral and Cranio-Maxillofacial, Ninth People's Hospital, School of Medicine, Shanghai Jiao Tong University, Shanghai 200240, China
c.
Department of Obstetrics, Shanghai First Maternity and Infant Hospital, Tongji University School of Medicine, Shanghai 201204, China

liujqmj@163.com

huaxiaolin_sh@163.com

haowei@sjtu.edu.cn

Received Date: 27 March 2019
Revised Date: 30 April 2019
Accepted Date: 6 May 2019
Available Online: 7 January 2019

Figures(4)

A novel channel-wall engineering strategy of the porous materials cationic covalent organic frameworks (COFs) is established based on rapid microwave-assisted anion exchange reaction and utilized to prepare a set of new COFs. Due to the interaction between the carbon dioxide (CO₂) and the acetate anion, the resulting SJTU-COF-AcO shows greatly enhanced carbon dioxide capacity up to 1.7 times of the pristine COF. The effect of the counter anions to CO₂ capacity in the cationic COFs is investigated for the first time, which demonstrates that our channel-wall engineering strategy is a promising way to tailor the property of COFs for high CO₂ capacity.
- Covalent organic framework,
- Channel-wall engineering,
- Carbon dioxide capture,
- Microwave-assisted synthesis,
- Anion exchange
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