Citation: Li Qin, Wang Xiaopei, Xiong Xueqing, Zhu Shuihong, Meng Zhaohui, Hong Yongying, Lin Changxu, Liu Xiangyang, Lin Youhui. Graphene-supported biomimetic catalysts with synergistic effect of adsorption and degradation for efficient dye capture and removal[J]. Chinese Chemical Letters, ;2020, 31(1): 239-243. doi: 10.1016/j.cclet.2019.04.039 shu

Graphene-supported biomimetic catalysts with synergistic effect of adsorption and degradation for efficient dye capture and removal

a.
Research Institute for Biomimetics and Soft Matter, Department of Physics, Fujian Provincial Key Laboratory for Soft Functional Materials Research, Xiamen University, Xiamen 361005, China
b.
Department of Physics, National University of Singapore, Singapore 117542, Singapore

^**

liuxy@xmu.edu.cn

linyouhui@xmu.edu.cn

Received Date: 16 February 2019
Revised Date: 2 April 2019
Accepted Date: 16 April 2019
Available Online: 18 January 2019

Figures(4)

Design and development of iron porphyrin-based artificial enzymes system have been attracting a lot of attention. Herein, without any toxic reductant and harsh processing, we present a facile one-pot method to fabricate bifunctional catalytic nanocomposites consisting of graphene and hemin by using vitamin C as a mild reduction reagent. The presence of graphene helps the formation of a high degree of highly active and stable hemin on the graphene surface in a monomeric form through their π-π stacking interaction. As a result, such nanocomposites possess a superior adsorption capacity and intrinsic peroxidase-like catalytic activity. Moreover, by the combination of their dye adsorption ability, RGOhemin nanocomposites can serve as a suitable candidate for efficient capture and removal of dyes via a synergistic effect. Our findings may pave the way to apply graphene-supported artificial enzymes in a variety of fields, such as environmental chemistry, bionics, medicine, and biotechnology
- Nanozymes,
- Pollutant removal,
- Solid matrix,
- Supported catalyst,
- Synergistic effect
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1.
沈阳化工大学材料科学与工程学院沈阳 110142