Citation: Xin Dai, Tong Liu, Ye Du, Jie-Yu Cao, Zhong-Juan Wang, Jie Li, Peng Zhou, Heng Zhang, Bo Lai. Synergistic effect in enhancing treatment of micro-pollutants by ferrate and carbon materials: A review[J]. Chinese Chemical Letters, ;2025, 36(8): 110548. doi: 10.1016/j.cclet.2024.110548 shu

Synergistic effect in enhancing treatment of micro-pollutants by ferrate and carbon materials: A review

Xin Dai ^{a, b} ,
Tong Liu ^{a, b} ,
Ye Du ^{a, b, *,} ,
Jie-Yu Cao ^{a, b} ,
Zhong-Juan Wang ^{a, b} ,
Jie Li ^{a, b} ,
Peng Zhou ^{a, b} ,
Heng Zhang ^{a, b} ,
Bo Lai ^{a, b, *,}

a.
College of Architecture and Environment, Sichuan University, Chengdu 610065, China
b.
Sino-German Centre for Water and Health Research, Sichuan University, Chengdu 610065, China

duyeah@scu.edu.cn

laibo@scu.edu.cn

Received Date: 29 May 2024
Revised Date: 8 October 2024
Accepted Date: 12 October 2024
Available Online: 13 October 2024

Figures(10)

Ferrate [Fe(Ⅵ)] has demonstrated its efficacy as a potent oxidizing agent in the treatment of wastewater, showcasing its potential for application in environmental remediation. The self-decomposition of Fe(Ⅵ) results in the formation of Fe(Ⅳ)/Fe(Ⅴ), which exhibits remarkable reactivity and selectivity towards the degradation of electron-rich micro-pollutants. Here we presented a comprehensive review on the removal of micro-pollutants in Fe(Ⅵ)/carbon materials (CMs) systems, encompassing an analysis of the oxidation mechanism and mutual activation, thereby providing guidance for the efficient elimination of recalcitrant micro-pollutants. The combnation of Fe(Ⅵ) and CMs can significantly enhanced the removal efficiency of various pollutants, with an increase ranges from 30% to 70%. The rate constants for pseudo-first order reactions were increased ranging from 3 to 14 times, while the total organic carbon (TOC) removal rate was effectively doubled. The presence of active species, including hydroxyl radicals, superoxide radical and Fe(Ⅳ)/Fe(Ⅴ) generated by Fe(Ⅵ) and CMs, can significantly enhance the oxidation efficiency of micro-pollutants which are not easily degraded solely by Fe(Ⅵ) or CMs. Furthermore, Fe(Ⅵ) can enhance the surface area and void volume of CMs, thereby reinforcing the adsorption capacity towards micro-pollutants.
- Ferrate,
- Carbon materials,
- Mutual activation,
- Oxidation mechanism,
- Reactive iron
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沈阳化工大学材料科学与工程学院沈阳 110142