Citation: Yuxue Mo, Liling Liao, Dongyang Li, Rongwu Pan, Yanhong Deng, Yanliang Tan, Haiqing Zhou. Development prospects of metal-based two-dimensional nanomaterials in lithium-sulfur batteries[J]. Chinese Chemical Letters, ;2023, 34(1): 107130. doi: 10.1016/j.cclet.2022.01.023 shu

Development prospects of metal-based two-dimensional nanomaterials in lithium-sulfur batteries

Yuxue Mo ^{a, b, e} ,
Liling Liao ^b ,
Dongyang Li ^b ,
Rongwu Pan ^d ,
Yanhong Deng ^a ,
Yanliang Tan ^{a, *,} ,
Haiqing Zhou ^{b, c, *,}

a.
College of Physics and Electronic Engineering, Hengyang Normal University, Hengyang 421002, China
b.
Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education, Key Laboratory for Matter Microstructure and Function of Hunan Province, Department of Physics and Synergetic Innovation Center for Quantum Effects and Applications, Hunan Normal University, Changsha 410081, China
c.
Hunan Joint International Laboratory of Advanced Materials and Technology for Clean Energy, Changsha 410082, China
d.
Hunan Shengli High-tech Energy Technology Co., Ltd., Yongzhou 425000, China
e.
Hunan Provincial Key Laboratory of Intelligent Information Processing and Application, Hengyang 421002, China

hytyl@163.com

hqzhou@hunnu.edu.cn

Received Date: 20 November 2021
Revised Date: 20 December 2021
Accepted Date: 9 January 2022
Available Online: 15 January 2022

Figures(8)

A lithium-sulfur (Li-S) system is an important candidate for future lithium-ion system due to its low cost and high specific theoretical capacity (1675 mAh/g, 2600 Wh/kg), which is greatly hindered by the poor conductivity of sulfur, large volume change and dissolution of lithium polysulfides. Two-dimensional (2D) materials with monolayers or few-layers usually have peculiar structures and physical/chemical properties, which can resolve the critical issues in Li-S batteries. Especially, the metal-based 2D nanomaterials, including ferrum, cobalt or other metal-based composites with various anions, can provide high conductivity, large surface area and abundant reaction sites for restraining the diffusion for lithium polysulfides. In this mini-review, we will present an overview of recent developments on metal-based 2D nanomaterials with various anions as the electrode materials for Li-S batteries. Since the main bottleneck for the Li-S system is the shuttle of polysulfides, emphasis is placed on the structure and components, physical/chemical interaction and interaction mechanisms of the 2D materials. Finally, the challenges and prospects of metal-based 2D nanomaterials for Li-S batteries are discussed and proposed.
- Lithium-sulfur battery,
- Two-dimensional materials,
- Cathode materials,
- Anode materials,
- Anode protection
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沈阳化工大学材料科学与工程学院沈阳 110142