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Citation: Jun Zhao, Hao Wu, Ke Xin Huang, Shu Yun Shi, Hua Peng, Xian Feng Sun, Liu Rong Chen, Qun Xiong Zheng, Qi Jun Zhang, Xiao Jiang Hao, Joachim Stöckigt, Xiao Kun Li, Yu Zhao, Jia Qu. One chloro-furoeremophilanoid and two new natural dimers from Ligularia atroviolacea[J]. Chinese Chemical Letters, ;2008, 19(11): 1319-1322. doi: 10.1016/j.cclet.2008.09.013 shu

One chloro-furoeremophilanoid and two new natural dimers from Ligularia atroviolacea

a Department of Traditional Chinese Medicine and Natural Drug Research, College of Pharmaceutical Sciences, Zhejiang University, Hangzhou 310058, China;
b Key Laboratory of Southern Zhejiang TCM R&D, Pharmacy School of Wenzhou Medical College, Wenzhou 325035, China;
c School of Chemical Engineering, Central South University, Changsha 410083, China;
d Kunming Institute of Botany, Chinese Academy of Sciences, Kunming 650204, China

Received Date: 7 April 2008

Fund Project: This work is by part financially supported by DAAD-CSC PPP project (No. CSC [2004] 3067) and intramural foundation from Wenzhou Medical College. We thank Prof. Zhong Jian Jia and Prof. Handong Sun for useful discussions. The authors are grateful to Dr. Shi Zhi Chen for the help of improving the biogenesis hypothesis.

Three new compounds,including one chloro-furoeremophilanoid (1),one eremophiladiolide (2),a rare dimer of nor-furoeremophilanoid,ligulatrovine A (3),and a known furoeremophilanolide (4),were isolated from Ligularia atroviolacea.The structures of compounds 1-4 were elucidated by spectroscopic methods including ID and 2D NMR experiments as well as X-ray diffraction study.
- Natural sesquiterpene,
- Eremophiladiolide,
- Dimer,
- Chloro-furanoeremophilane,
- X-ray,
- Ligularia atroviolacea
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